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The phrase "unwind by" is grammatically correct and commonly used in written English.
It is typically used to describe an activity or method of relaxation or destressing. Example: After a long day at work, I like to unwind by taking a hot bath and reading a good book.
Exact(43)
Beljan used to unwind by riding motorcycles.
"And so some guys after games may unwind by stopping at a bar.
One summer afternoon, the governor tried to unwind by taking a swim in the pool.
He used to unwind by spending hours listening to music, any kind of music.
Most evenings after work, I unwind by taking my miniature poodle for a walk around my neighborhood.
They spend their days hooking and hoisting — even when off-duty, since a number of them unwind by going fishing.
Similar(17)
Similar smFRET histograms and periodic unwinding time traces were obtained, implying that the periodic G4 unwinding by a Pif1 monomer may be general and not specific to sub-species of G4 structures.
He unwinds by watching sitcoms and sports on television.
He also unwinds by strolling over the Henry Hudson Bridge to Manhattan's 196-acre Inwood Hill Park, where he enjoys exploring for old ruins now overtaken by tulip trees.
The stockmarket's fall is made worse by the increased unwinding by big banks (some of the biggest holders of shares) of cross-shareholdings in other companies.
Some other bits of local color: episode titles are taken from Elvis Presley songs, and Hendricks unwinds by taking to a nightclub stage and doing his own covers of the King.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com