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The phrase "opt to undertake" is correct and usable in written English.
It means to choose or decide to do something. Example: After carefully considering all of my options, I have opted to undertake the project on my own.
Exact(4)
You can then opt to undertake the exercises Mackendrick set his students, or proceed to the comparison of two drafts of a scene from Success.
At some medical schools, students can opt to undertake a 1 year intercalated degree, usually a BSc, in addition to their medical course.
Sixty seven (22.9%) students already had a first degree and this was the primary reason why they did not opt to undertake an intercalated degree.
At the end of the 26-week follow-up period the participant may continue their treatment as per local policy and for control participants, may opt to undertake one of the trial treatments if indicated and appropriate for them at that time.
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Vosshall opted to undertake her first clinical trial.
The DOE has instead opted to undertake research to develop new cycles that "burn" the radioactive waste.
Milford opted to undertake training in ordnance in England after the war, and also became married at this time.
The rise in tuition fees is likely to result in substantially fewer medical students opting to undertake an intercalated degree.
Over the last few years the numbers of students who have opted to undertake an intercalated degree have been steadily decreasing despite the advantages in securing foundation posts.
Since the required sample represented most of the eligible patients, we opted to undertake a "whole population" study and invited all practices and eligible patients.
Furthermore, the rise in tuition fees is likely to result in substantially fewer medical students opting to undertake an intercalated degree, threatening to further reduce the number of doctors following an academic path.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com