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"volatile personality" is correct and usable in written English.
You can use it to refer to someone whose behavior is unpredictable, often prone to rapid changes in mood or emotion. For example: "I would not recommend hiring her as a manager because of her volatile personality."
Exact(42)
So Milbury, with a volatile personality, has increased the volatility around his franchise.
Augustine had this deep, volatile personality.
Once again, Mike Milbury has demonstrated his volatile personality".
His volatile personality and opinions were captured in his autobiography, Beneath the Underdog, published in 1971.
She had many friends and admirers, but had also generated enmity because of her volatile personality.
And the defense put several witnesses on the stand who testified to Mr. Black's volatile personality.
Similar(18)
Ms. Kaufman suggested Robert DeNiro -- a specialist in volatile personalities.
Mr. Snyder and Mr. Davis, both volatile personalities, had a famously stormy relationship.
They rarely gamble on volatile personalities, though they will make the occasional exception (see Stephen Jackson).
You think primarily of designers with big, brash, occasionally volatile personalities.
She wasn't looking for volatile personalities, in the way of a reality-television producer; it was more like finding roommates to share an apartment.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com