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Discover LudwigThe word 'unlimitedly' is not correct in written English
It is not an accepted term. You could use the phrase 'without limitation' or 'without bounds' instead. Example sentence: She was determined to reach her goals without limitation.
Dictionary
unlimitedly
adverb
In an unlimited way.
synonyms
Exact(2)
He said later that he wanted his language to be "unlimitedly rich, flexible, full of every 'bagatelle' that gives life to language," but, above all, he wanted it to be easy to learn, and that is how he promoted it.
According to classical physics the intensity of this continuous radiation would grow unlimitedly with growing frequencies, resulting in what was called the ultraviolet catastrophe.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com