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Epithelial basement membrane and extracellular matrix (ECM) are composed of tough network of fibrillar ECM proteins that can be directly degraded only by divalent cation-dependent matrix metalloproteinses (MMPs).
Upon photocrosslinking, flexible and tough networks with excellent elastomeric properties were obtained.
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Haque, M. A., Kurokawa, T. & Gong, J. P. Super tough double network hydrogels and their application as biomaterials.
In this study, ionoprinting has been combined for the first time with a tougher interpenetrating network polymer (IPN) hydrogel with dual pH and temperature responsiveness.
Tough double network (DN) hydrogels are a kind of interpenetrating network (IPN) gels with a contrasting structure; they consist of a rigid and brittle 1st network with dilute, densely cross-linked short chains and a soft and ductile 2nd network with concentrated, loosely cross-linked long chains.
These relationships may be utilized to design tough photopolymerizable networks for use in mechanically rigorous biomedical applications.
Webber, R. E., Creton, C., Brown, H. R. & Gong, J. P. Large strain hysteresis and Mullins effect of tough double-network hydrogels.
