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The phrase "to ally" is correct and usable in written English
It can be used when referring to the act of forming an alliance or partnership with someone or something. Example: "The two countries decided to ally in order to strengthen their defense against common threats."
Dictionary
to ally
verb
To unite, or form a connection between, as between families by marriage, or between princes and states by treaty, league, or confederacy
synonyms
Exact(59)
Likud chose instead to ally itself to smaller parties.
By teatime he had been downgraded to "ally".
After the Soviet invasion, Muslim leaders were eager to ally themselves with the Afghan resistance.
Disappointed claimants would almost certainly try to move up the corporate ladder to Ally for payment.
The French luxury companies have seized the opportunity to ally with Italian savoir-faire.
That is what tempts governments and security forces to ally themselves with vigilantes.
The logical thing would be for two blocs to ally, but instead that's not happening".
Otherwise it may be tempted to ally with the rich to block reform.
But for now they chose to ally themselves with a more unsavoury icon.
Through the 20th century, liberal Republicans and Democrats tended to ally against conservative Republicans and Democrats.
Similar(1)
A Shivga extraordinaire: a go-to ally and friend!
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Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com