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The phrase "the largest amount of" is correct and usable in written English.
You can use this phrase to refer to a large quantity or amount of something. For example, "The donation drive collected the largest amount of money ever seen in this city."
Exact(60)
In the Northwest, the largest amount of green power comes from hydroelectricity.
It was the largest amount of money although it wasn't physically that big.
Russia has the most nuclear weapons and the largest amount of fissile material in the world.
Under the settlement, each borrower will receive about $125,000, the largest amount of relief.
"The largest amount of contract awards comes in this last fiscal quarter, which ends in September.
This enabled the robbers to pick the appropriate day to secure the largest amount of cash.
It is the largest amount of foreign assets ever seized in an American sanctions action.
The largest amount of rain, 6.2 inches, fell in Edgartown, Mass., on Martha's Vineyard.
Undoubtedly, however, the largest amount of material was written in Greek.
"The groups with the largest amount of people receive less fish per person," Mr. Hoover said.
Xmax denotes the largest amount of data.
More suggestions(18)
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com