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It is shown that the model predicts the effect of variations in solids inventory well.
High solids circulation, very low solids residence time and low solids inventory are observed during operation.
The obtained residence time, in combination with the solids inventory, determined the solids circulation for a particular batch experiment.
Furthermore, it is shown that with the applied kinetics data, the OC is only fully oxidized in the AR when the AR solids inventory is much larger than the FR solids inventory or when both reactors are very large.
Model simulations showed that the reactor temperature, the solids circulation flow rate and the solids inventory were the most relevant operating conditions affecting the oxygen demand.
The kinetic model was used to calculate the solids inventory needed in the fuel reactor for complete combustion of three different rank coals.
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The minimum solids inventories depended on the fuel gas used, and followed the order CH4>CO>H2.
And its effects on the flow behavior are studied by investigating the variation of axial voidage profile and solids flux in the riser under different solids inventories.
It was found that the circulation rates and the solids inventories are linked, and the possible operating conditions are closely dependent on the reactivity of the OCs.
Moreover, a plot to calculate the solids inventories in a CLC system, valid for any type of OC and fuel gas, is proposed.
Thus, both the internal circulation in the fuel reactor, and the circulation between air and fuel reactor, could be varied in a large range with only minor impact on the solids inventories of the air and fuel reactors.
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