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Discover LudwigThe phrase "simplest of" is correct and usable in written English.
It can be used to refer to something that is the most basic or uncomplicated among a group or category. Example: "Among all the solutions we discussed, the simplest of them is to just follow the original plan."
Exact(58)
The simplest of group activities were responsible.
Jones took the simplest of catches.
He couldn't understand the simplest of instructions.
Messi tacks right and brushes past, the simplest of shuffles.
It's the simplest of the three works, but elegantly simple.
It is also, by far, the simplest of the three.
The simplest of salads, but a rather luxurious one nonetheless.
Clearly, I have stuck to the simplest of the simple.
Transport is among the simplest of our problems to solve.
Mastering the simplest of human activities remain formidable challenges.
The simplest of these is the familiar solvent benzene.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com