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Discover LudwigThe phrase "set off on" is correct and usable in written English.
It is typically used to mean starting something, usually a journey or a course of action. For example: The travellers set off on their adventure across Europe.
Exact(60)
The one time he set off on a run Nathaniel Clyne caught and dispossessed him.
We set off on foot.
I set off on my scooter.
So he set off on foot.
They then set off on the trail back toward civilization.
So Barker said he set off on foot.
Then we set off on the long, lovely drive.
The 12-member group set off on Saturday.
Leon set off on a world tour of cacti hotspots.
Groups set off on foot towards the south and east.
And, in fact, she has set off on her climb.
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Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com