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The phrase "set her heart" is correct and can be used in written English.
It is typically used in phrases such as "The moment she saw him, her heart was set on marrying him". This phrase is typically used to express strong feelings of love and devotion.
Exact(34)
By age 11, she had set her heart on studying enology.
To think that the Jewish Montessori was once the school Kate had set her heart on!
Despite applying for the job herself, she never set her heart on it.
When she was seven, Wu Ying set her heart on a pair of long-haired rabbits.
So did she set her heart on DJing at an early age?
Switzer has set her heart on persuading the International Olympic Committee to include the event in the next games.
Similar(26)
She lived in South America, Spain and Australia before returning to Britain and setting her heart on becoming a midwife.
To be exact, Mr. Turetsky, a fireplug of a man, gave her a bear hug that had the startling effect of setting her heart aflutter.
Smitten Ester walks out on her boyfriend and sets her heart on a future with Rask who, frustratingly, has yet to make a move.
Not surprisingly, that's the path followed by the film's protagonist, a young Saudi girl (Waad Mohammed) called Wadjda who sets her heart on buying a new bicycle.
As we well know, a girl's capabilities are endless and she is fully equipped to do whatever she sets her heart and mind to.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com