It is noteworthy that the reconstruction using the latest gate (t = 2.8ns) results in the most accurate quantification and the least crosstalk for the compound with the longer lifetime, implying the necessity of the late gates for effective separation of the objects with lifetime contrast.
Given polarized excitation and single detection channel at magic angle conditions (54.7°) separation of species with the same lifetime is impossible.
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It was reported that the wave function overlap integral is inversely proportional to the radiative lifetime [16], giving rise to the charge separation of the electron and hole for longer lifetime values.
As opposed to H2 line emission, where the line width is small compared to the separation of the individual lines, the short lifetime of the super-molecule results in line widths large enough that they merge into a continuum.
During PEC water splitting, the BiVO4 acts as the primary light absorber for wider solar spectral harvesting, and the ZnO prompts the transfer of the photo-excited high-energy electrons, which would render them with prolonged lifetime and enhanced separation of the photogenerated charge carriers.
The successful separation of FRETing and nonFRETing donor species based on lifetime contrast similar to previously reported lifetime based tomographic studies in vivo [ 43, 44] indicates the feasibility of this approach for FRET imaging in live animal models.
The result suggested a more efficient separation and longer lifetimes of photoexcited electron hole pairs.
It clearly showed that the photocurrent response of these three samples was NT > NFs > Mix, indicating a more efficient separation and longer lifetimes of electron-hole pairs in Sn-Ti NT than NF and Mix samples.
The photocurrent response and EIS results demonstrated that a much more efficient separation and longer lifetimes of electron-hole pairs existed in Sn-Ti nanotube, which should be responsible for the increased photocatalytic activities.
