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The phrase "relationship deteriorate" is correct and usable in written English.
You can use it to describe relationships that are becoming worse with time, such as, "As the years passed, their relationship deteriorated."
Exact(6)
Should that relationship deteriorate, the chances of a deal with the Palestinians on the same basis will recede.
Similarly, Turkey and Iran are backing different sides in Syria, but neither will let their bilateral relationship deteriorate too sharply; Iran needs Turkey to go easy on enforcement of sanctions, and Turkey needs Iran to continue selling its natural gas.
Should the relationship deteriorate, it is more difficult to get rid of a co-tenant whose name is on the lease than someone who has signed only a roommate agreement.
At a joint news conference after their meeting, both Mr Kerry and Mr Lavrov said the US and Russia needed to cooperate and could not let the relationship deteriorate.
But given the hostility that Mexico perceives from the United States, Peña Nieto has little choice politically but to let the relationship deteriorate.
New limits may make the quality of a relationship deteriorate, and may also cause the couple to suffer more as a whole.
Similar(52)
Once I started writing, though, our relationship deteriorated.
Their relationship deteriorated when he was a teenager, but they eventually reconciled.
Had their relationship deteriorated to the point where it was irreparable?
But afterwards our relationship deteriorated because Tony stopped communicating with me".
But the relationship deteriorated this season, something that Mike Mussina of the Yankees noticed from afar.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com