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From now on, this manuscript is focused on IL-related phonon self-energy renormalizations.

All authors contributed to and commented on this manuscript.

We thank S. L. Pfirman for guidance on this manuscript.

We thank Lisa Roux for comments on this manuscript.

The authors thank Kenneth L Baughman for advice on this manuscript.

We thank members of the Todd lab for input on this manuscript.

We thank R. Pillai and E. Heard for comments on this manuscript.

HF was supported by an Australian Government Research Training Program Scholarship while working on this manuscript.

We highly appreciate the anonymous reviewers for their constructive comments on this manuscript.

We are also grateful for the comments on this manuscript by K. Zhang.

JA was supported by an Australian Research Council Professorial Future Fellowship while working on this manuscript (Grant FT140100195).