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The database, together with adjoint based sensitivity and uncertainty tools for transmutation systems developed to quantify the importance of nuclear data on nuclide concentrations, are described.
A nested-sampling design was used to test for effects of increasing catchment scale on nuclide concentrations with upstream catchment areas ranging from 4 to 130,000 km2.
In this study, a novel, systematic determining method was proposed based on nuclide decay, radon diffusion migration theory, and the mass conservation law, and an associated experimental device was designed and manufactured.
The analytical solution to the nuclide concentrations at the fracture outlet is governed by nine parameters representing different mechanisms acting on nuclide transport through a fracture, including diffusion into the rock matrices, diffusion into the stagnant water zone, chain decay and hydrodynamic dispersion.
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As its fathers, grandfathers, and so on each decay exclusively to one nuclide, this gives only one possible way for the starting nuclide in the neptunium series (neptunium-237) to decay – via eventual production of astatine-217.
A valid performance assessment of radioactive waste repositories strongly depends on the reliability of nuclide transport parameters, including distribution and diffusion coefficients.
At present several accelerator manufacturers offer production packages for these radionuclides emphasizing targetry with consideration of the cyclotron extracted energies for nuclide production and on-line chemistry systems for the continuous production of specific precursors or radiotracers.
The diffusion dialysis coefficient had a negative effect on the removal of nuclides, but had no significant effects on the removal of boron.
It is expected to be used for the treatment of nuclide transport of a decay chain for safety assessment, as well as for design feedback on the KRS both on a deterministic and a probabilistic bases.
Another advantage is that the developed system is independent on the nuclide used and can be used for any positron emitting tracer as shown in the present study.
We have been developing a web-based tool (WebCN) to calculate surface exposure ages and erosion rates based on the nuclide concentrations measured by the accelerator mass spectrometry.
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Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com