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The phrase 'most frequent users' is correct and can be used in written English.
It usually refers to people who use a particular service or product most often or most regularly. For example, "Loyalty rewards are offered to the company's most frequent users."
Exact(60)
Pharmaceutical companies are the most frequent users of selection invention.
*The most frequent users tend to live in the Northeast and have large families.
Patients with chronic conditions are often the most frequent users of health care.
Older adults have high rates of health problems and are the most frequent users of healthcare.
Still, users of the unlimited cards are, almost by definition, the most frequent users of mass transit.
The most frequent users appear to be China as an attacker and the U.S. as the attacked.
The number of households using a charity at least once a week has increased by 500,000 since 2014, with single parent households being the most frequent users.
What had once been a useful tool for wishing away anything inconveniently addressed by mainstream media – like recorded history – turned on its most frequent users.
Direct marketers, the most frequent users of the technique, say it is akin to the standard practice among Internet advertisers of tracking which banners Web surfers click on.
Executions in the United States, usually among the world's most frequent users of the death penalty, dropped to 42 in 2007, the lowest.
The Web search service Google has quietly started placing a counter on its home page for a small number of its most frequent users.
More suggestions(15)
most regular users
most common users
most frequent seekers
most frequent service
most frequent irritants
most frequent targets
most frequent travelers
most frequent contacts
most frequent culprits
most frequent phenomena
most frequent churchgoers
most frequent manifestations
most psychedelic users
most low users
most frequent visitors
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com