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Discover LudwigThe phrase "largest percentage" is correct and usable in written English.
It is typically used when comparing two or more percentages to indicate the largest one. For example: "The northern region had the largest percentage of rainfall last month, at an average of 8 inches."
Exact(58)
The largest percentage increase occurred at the high school level.
These were the largest percentage increases in the entire conflict.
"The largest percentage -- about 70percentt -- is mine," he added.
Mississippi has the largest percentage of black residents, at 37%.
The largest percentage -- 46percentt -- fell in the category of "haven't heard enough".
And lending dropped by the largest percentage since the government began collecting data in 1984.
So the largest percentage winner — no matter how small — would become the president.
The fall in live births in 2013 represented the largest percentage annual decrease since 1975.
It was the largest percentage margin of victory for a Republican in the city's history.
Under the current system, too, the largest percentage winner normally becomes President.
Hepatitis C patients make up the largest percentage of people requiring liver transplants.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com