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Smooth critical locus linking between the critical points of pure water and ammonia was obtained.
The critical locus showed a good agreement with the most reliable experimental data.
Stability theory for multicomponent fluid mixtures is used to calculate the spinodal and the critical locus for a multicomponent mixture.
The tangent plane global stability tests are included to locate UCEPs and LCEPs which are intersections of the critical locus and the LLG line.
Such transitions marked by the existence of a turning point in the critical locus are commonly found in type III and IV mixtures.
The Gibbs minimization performs better than the fugacity method in locating phase equilibria in the vicinity of the critical locus of the mixtures.
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Unusual branches of critical loci were found with WS and MHV2 mixing rules.
A robust method for this task is certainly a powerful tool for calculation of critical loci.
Far away from the critical loci of the mixtures all the three methods are found to be equally reliable.
Methods are described for the prediction of critical loci, upper and lower critical end points, and azeotropic lines in binary and multicomponent mixtures.
In this work, the H2 group is added to the well-established PPR78 model in order to predict mutual solubility and critical loci of hydrogen-containing systems.
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