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"create a repertoire" is correct and usable in written English.
You can use this phrase to refer to creating a collection of skills, experiences, or knowledge. For example, "Gail plans to create a repertoire of marketing strategies in order to advance her career."
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In one of the several film clips presented during the evening, he paid tribute to the generosity of the philanthropist Irene Diamond, who died in 2003, and he stated his goal for the institute: "to create a repertoire for the times in which we live".
Because of the diversity of PDZ domains, this opens avenues for the design of related phosphoswitchable domains to create a repertoire of regulatable interaction parts for synthetic biology.
Shane tried to create a repertoire for these groups that included both the older and expected Kingston Trio standards like "Tom Dooley" and "M.T.A".
Originally, three choreographers were asked to create a repertoire based on Graham's famous solo, Lamentation, that was to last for less than four minutes and be crafted, from start to finish, in 10 hours of rehearsal.
Repetitive DNA was identified and annotated in SOAP assembled genomes of the four isolates described above to create a repertoire of repeats specific to the Zymoseptoria genus using the REPET pipeline (Flutre et al. 2011).
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With David writing the lyrics and Don taking care of the music, the pair recruited the R&B singers Harry Bowen and Sweet Pea Atkinson and set about creating a repertoire that, Don declared, would sound "like the Motown revue on acid".
"From planning State Dinners that paid tribute to world leaders such as Nelson Mandela to creating a repertoire of First Lady Lunches to orchestrating barbecues for thousands of guests on the South Lawn, I was thrilled to help shape White House cuisine and events for more than a decade".
As reviewed elsewhere, the need to suppress exacerbation of the endogenous infections creates a repertoire of highly reactive effector memory, which are potentially autoreactive.
The observed gene duplication within the bovine TRB locus has created a repertoire of phylogenetically diverse functional TRBV genes, which is substantially larger than that described for humans and mice.
Most vertebrate species utilize antibody and T-cell receptor (TCR) genes to create a vast repertoire of antigen sensor molecules on their B and T lymphocytes, respectively.
Plants, as sessile organisms, evolve and exploit metabolic systems to create a rich repertoire of complex natural products that hold adaptive significance for their survival in challenging ecological niches on earth.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com