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The phrase 'constituted the largest' is correct and can be used in written English.
You can use this phrase to talk about a group or amount that is larger than any others. For example: "The group of students from America constituted the largest number of attendees at the conference."
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Spanish males, who constituted the largest group of immigrants, freely intermarried with indigenous women and Africans.
They constituted the largest number of Japanese to visit here since Soviet soldiers expelled the last Japanese inhabitants in 1949.
"In many large evangelical congregations," the researchers wrote, "the participants constituted the largest thoroughly integrated gatherings we have ever witnessed".
"This urban and rural landscape, linked by road and canal networks, now seems to have constituted the largest empire on earth in the 12th century," Sharrock said.
In 2007, the United Nations Foundation said that efficiency improvements constituted "the largest, the most evenly geographically distributed, and least expensive energy resource".
Muskogean-speaking peoples constituted the largest linguistic group in the aboriginal Southeast and minimally included the Choctaw, Chickasaw, Apalachee, Creek, Seminole, Alabama, Koasati, Hitchiti, and Mikasuki branches.
It was the Mets' ninth consecutive loss to the reigning National League East champions, and many of the 56,350 who constituted the largest home-opener crowd in franchise history left in waves after the eighth.
Officials from the organization said they believed that this week's event in Los Angeles constituted the largest free health care event in the country, with the arena and all supplies and services provided free to the group.
Darius' campaign against the Greeks, in 490, and, after his death, that of his son Xerxes, in 480-479, constheuted the largest military undertakings in history up to that point.
Because the market for residential mortgages and the mountain of securities built on them constituted the largest financial market in the world, that regulator probably would have kept a watchful eye on it.
Therefore, it appeared that the sodium oxide constituted the largest amount among all impurities.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com