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Binary interaction parameters are calculated from experimental PTxy data and generalized correlations are proposed.

It is shown that three binary interaction parameters are sufficient to correlate each binary system.

The increased miscibility is quantitatively predicted by the modified theory when binary interaction parameters are calculated by group contribution methods.

When all binary interaction parameters are zero, these parameters are calculated analytically, otherwise this equation is an approximation and the three mentioned constants are calculated from curve fitting (Leibovici et al. 1996).

The comparison reveals that on average the most accurate VLE and density predictions are obtained with the SAFT-based EoSs, while similar results in VLE calculations are obtained with the four EoSs when regressed binary interaction parameters are used.

The E-PPR78 model is a predictive version of the widely used Peng Robinson equation of state in which the binary interaction parameters are estimated by a group-contribution method.

Also, the corresponding binary interaction parameters were regressed.

Initially, new binary interaction parameters were estimated for (CO2 + glycol) binary mixtures.

To construct the theoretical phase diagrams, all binary interaction parameters were determined accurately and thoroughly revisited.

The binary interaction parameters were adjusted, and the volume translation technique was employed to correlate the experimental compositions and densities.

To improve the predictions, the binary interaction parameters were adjusted and the volume translation technique was applied.