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As well the correlations between char structure and surface area to char reactivity were examined.
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The calculated results reveal the relationship between the char structure and the char reactivity.
The relationship between the char structure and the gasification reactivity has been the subject of only few researches (Barziv et al. 2000; Zaida and Sheng 2007).
The higher the quantity, the higher is the thermal stability of the char residue and the more compact and porous char structure may be the main reasons for the phenomenon above.
The changes in char reactivity during the reactions with steam or oxygen were mainly attributed to the Na content and the char structure.
The thermally stable biochar provided a compact char structure during combustion which prevented the heat and mass transfer between the polypropylene and the ambient O2.
The elementary reactions of the char gasification and volatile char interactions, which are consist of the adsorption of free radicals from volatiles, the volatilisation of catalyst and the evolution of char structure affected by radicals from volatiles, were proposed.
Our results have clearly shown that volatile char interactions can lead to drastic decreases in char reactivity due to the volatilisation of Na and the changes in char structure.
The extent of which would rely on the specific char structure, such as the carbon functional groups and ordering degree.
To explore the variety of char structure features, the Scanning Electron Microscope (SEM) and Raman Spectrometer are adopted.
A lower ID/IG ratio implies higher graphitization degree and thermal stability of the char structure [22, 66].
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