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The phrase "as their last" is correct and usable in written English.
It can be used in contexts where you are referring to something being done or given as a final act or item.
Example: "He decided to write a heartfelt letter to his family as their last communication before leaving."
Alternatives: "as their final" or "as their ultimate".
Exact(60)
The military should view a service member's potential transition as their last and most lasting mission.
So they tend to come to God as their last resort.
As tense as their last meeting was, they managed a joke between them on Monday.
As their last song ends and the duo make their exit, the audience bay for more.
For these users, the IT department is only as good as their last call to the Help Desk.
Clinton supporters are seizing on this story as their last lifeline of hope.
Most are incredibly sick and see us as their last beacon of hope.
GBV's fifth album, 1992's Propeller, was intended as their last.
Many of the students take Haqqani as their last name when they leave the madrasa.
Many saw today's auction as their last chance to make an independent nationwide network.
As their last moments slip away, they seem suddenly all the more sweet.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com