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"ancient of" is not a correct or commonly used phrase in written English.
It is possible that it may have been used in older texts or poetry as a poetic or archaic way of referring to something or someone very old or ancient. Example: "The ancient of the castle stood tall and proud, a testament to the rich history of the land." (Note: This example uses "ancient of" as a way to describe the castle, but it is not a commonly used phrase in modern English.).
Exact(59)
They represent most ancient of municipal traditions.
Ancient of Days, bless the innocent.
"It is the most ancient of stories".
Salt is also ancient, of course.
The Breadman was saying, "It is among the most ancient of grains.
He practices the most ancient of medical arts, the laying on of hands.
Most ancient of all are the Jack Hills, inland north-east of Geraldton.
(smash reinvention of the most ancient of TV formats, the game show).
Subject: William Blake (1757- 1827), author of The Marriage of Heaven and Hell, engraver of The Ancient of Days.
Cortona, which James calls "the most sturdily ancient of Italian towns," is even more narrowly up-and-down than Perugia.
The Successor by Ismail Kadare translated by David Bellos Canongate £9.99, pp207 Albanians are descended from the most ancient of European races, the Illyrians.
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Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com