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The phrase "ambitious new chapter" is correct and usable in written English.
It can be used to describe a significant and hopeful phase or development in a person's life, organization, or project.
Example: "After years of hard work, she is ready to embark on an ambitious new chapter in her career."
Alternatives: "bold new phase" or "exciting new journey".
Exact(1)
The US venture is an ambitious new chapter for the retailer, which began life in 1969 as a single shop in Dublin under the name Penneys – the name it still trades under in Ireland.
Similar(59)
"Working in the White House on a Saturday afternoon had become routine for Zeke Emanuel and Bob Kocher, Steven Brilll tells us at the beginning of Chapter 9 of his ambitious new history of the Affordable Care Act, "America's Bitter Pill" (Random House): But they were usually able to leave at a decent hour.
The latest chapter in the Norwegian capital's development is the ambitious new Ekeberg Sculpture Park that opens Sept. 26, the passion project of Christian Ringnes, a local real estate tycoon who bought the adjacent Ekeberg restaurant and donated tens of millions to create the park.
It's a new chapter.
A new chapter began.
For "new chapter," read "special relationship".
"Yesterday a new chapter started," Gimelstob said.
"She had a new chapter," Roger Peltzman said.
He called it a "new chapter".
"Having exceeded even the crazy ambitious goals we dreamed of for Android – and with a really strong leadership team in place – Andy's decided it's time to hand over the reins and start a new chapter at Google.
Today marks a new chapter".
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com