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The phrase "although the majority of" is correct and usable in written English.
It can be used to introduce a contrast or exception regarding a large group or number of people or things.
Example: "Although the majority of the participants agreed with the proposal, a few raised significant concerns."
Alternatives: "even though most of" or "despite the fact that most of".
Exact(60)
Although the majority of these mutations affected the R882 position, additional mutations were identified.
Although the majority of papillary thyroid cancer (PTC) is indolent, a subset of PTC behaves aggressively despite the best available treatment.
Although the majority of subepithelial lesions are benign, GI stromal tumors have malignant potential, making a definitive diagnosis important.
Although the majority of its articles pertained to Central Basin, News Hawks also promoted other subjects.
Although the majority of those attending are women, men come too.
Although the majority of the data were collected as described above, there were some exceptions.
Although the majority of cysts are benign, several varieties may be malignant or precancerous.
Although the majority of the general population decides not to offend, a significant proportion decides otherwise.
Species-specific differences existed, although the majority of the assemblage was considered to be urban-sensitive.
Although the majority of headpiece domains bind actin, there are some that lack this activity.
Although the majority of the musicians depicted are men, a significant number of female guitarists also appear.
More suggestions(16)
although the predominance of
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although the generality of
although the minority of
although the margin of
although the bulk of
although the part of
although the most of
although the progression of
although the influx of
although the content of
although the possibility of
although the maintenance of
although the history of
although the science of
although the condition of
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com