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The phrase "air of disquiet" is correct and usable in written English.
It can be used to describe a feeling of unease or anxiety in a particular situation or environment.
Example: "As the meeting progressed, an air of disquiet settled over the room, making everyone feel uneasy about the decisions being made."
Alternatives: "atmosphere of unease" or "sense of discomfort".
Exact(3)
Despite an enduring air of disquiet, the cumulative effect, choreographed by the sculptor's exceptional aesthetic sensitivity, is one of celebration.
Despite the air of disquiet, Timbers, who talks like a cool high-school teacher lots of vocal fry, the repeated use of "awesome"—addressed the cast with rousing enthusiasm.
And to add to the general air of disquiet, there seems to be - unless I am imagining this - a silent, fleeting cameo at the very beginning by Ian Brown, late of the Stone Roses, glimpsed morosely on his own in a pub called the Leaky Cauldron.
Similar(57)
The Book of Disquiet Fernando Pessoa, trans.
That will cause a lot of disquiet.
A vague sense of disquiet began to steal over me.
They usually arise out of disquiet, a sense of unease.
It has an element of disquiet and surprise.
And yet a shadow of disquiet hangs over her.
There was a lot of disquiet in that room".
In the mountains, too, there are signs of disquiet.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com