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The phrase "additionally a significant portion" is correct and usable in written English.
It can be used when introducing extra information that emphasizes the importance or size of a part of a whole.
Example: "Additionally, a significant portion of the budget will be allocated to research and development."
Alternatives: "furthermore, a considerable amount" or "in addition, a large segment".
Exact(1)
Additionally, a significant portion of survivors report inadequate screening for general health maintenance issues.
Similar(59)
Althaus [49], however, pointed out additionally that BEV charged with electricity with a significant portion of nuclear energy will be associated with a backpack of nuclear waste production.
Additionally, the hydrologic cycle of the Amazon basin has been shown to be unique, recycling a significant portion of its own precipitation from evaporation in the same basin [16].
But a significant portion probably did not.
So a significant portion is delegated to innovative technology.
A significant portion of Chaleur Humaine is about gender identity.
Undoubtedly, work will take a significant portion of these hours.
(The intelligence agency outsources a significant portion of its work).
But a significant portion of the cinematic city goes unsung.
"A significant portion of our people do not make it".
A significant portion of nonsubsective adjectives violate this assumption.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com