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The phrase "act of exasperation" is correct and usable in written English.
It can be used to describe a behavior or action that is driven by frustration or annoyance.
Example: "After hearing the same complaint for the third time, she let out a loud sigh, an act of exasperation that spoke volumes."
Alternatives: "gesture of frustration" or "display of annoyance".
Exact(2)
One way to interpret the hearing for Mr. Hossain was as an act of exasperation.
Earlier this month, in what looked very much like an act of exasperation, the chair of the UK's fake news enquiry, Damian Collins, flew his committee over the Atlantic to question Facebook, Twitter and Google policy staffers in an evidence session in Washington.
Similar(58)
Dr. Smalley's final response has an air of exasperation.
— Stephen Stills, 1966 The right-wing campaign to sabotage the Affordable Care Act has driven a lot of normally temperate people past the edge of exasperation.
He expressed the same degree of exasperation.
Yet this remains a source of exasperation.
I feel a familiar touch of exasperation.
Others detect a sly note of exasperation.
IT WAS a deliciously French moment of exasperation.
"No," Markieff said with a hint of exasperation.
In a brief interview, he showed a flash of exasperation.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com