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The phrase "a much more ambitious" is correct and usable in written English.
It can be used when comparing the level of ambition of one thing to another, indicating that it is significantly greater.
Example: "The new project is a much more ambitious undertaking than our previous initiatives."
Alternatives: "far more ambitious" or "significantly more ambitious".
Exact(60)
But she had a much more ambitious agenda.
Overnight, OWN had become a much more ambitious endeavor.
But a much more ambitious effort is needed.
In 1971, a much more ambitious recreation of the illustrations was begun [seen here].
Across the continent in Chile, a much more ambitious project could eventually come to fruition.
Now it is having to do so again, with a much more ambitious plan.
The House passed a much more ambitious and costly jobs bill in December.
The second edition was a much more ambitious work in both length and scope.
The workers are urging Amazon to adopt a much more ambitious effort.
But, following the second world war, his successors developed a much more ambitious agenda.
Emergency action is needed on a much more ambitious scale than is now being planned.
More suggestions(15)
a much more extensive
a significantly more ambitious
a considerably more ambitious
a much more daring
a much more comprehensive
a much more high
a much more courageous
a much more massive
a much more aggressive
a much more challenging
a much more exacting
a much more forward looking
a much more stable
a much more controllable
a much more apt
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com