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The phrase "a definite alignment between" is correct and usable in written English.
It can be used when discussing a clear or specific relationship or agreement between two or more entities or concepts.
Example: "There is a definite alignment between the company's goals and its marketing strategy, ensuring a cohesive approach to growth."
Alternatives: "a clear connection between" or "a specific correlation between".
Exact(1)
The story is invented, but there's a definite alignment between his emotional and mental life and mine".
Similar(59)
But the initial encounter between the designers and the artist had a definite element of surprise.
There was a definite kinship between Tarkovsky and Lennon.
They could not make a definite link between his condition and the explosion.
There is a definite kinship between Schubert's hurdy-gurdy player and Dylan's tambourine man.
In the past, Wilde said, there was also a definite division between the types of archers.
There is, however, a definite difference between the two as works of theater.
There's a definite spark between them, but it's clear this is only a reprieve.
Furthermore, doctors will tell you that there is a definite relation between anger and ulcers.
There's a definite lag between the time you tap and the time the screen responds.
Such an excitation behaves like a particle and therefore has a definite relationship between its energy and its momentum.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com