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Discover Ludwig"Most crucially" is correct and can be used in written English.
It is typically used to emphasize the most important aspect of a sentence or argument. Here is an example: "Most crucially, we must address the issue of climate change in order to ensure a sustainable future for our planet."
Exact(60)
Most crucially, it looked to the future.
Most crucially, people must stop buying ivory.
Most crucially, how should they be arrayed?
Most crucially, funding comes down to relationships.
Most crucially, of course, he was white.
Most crucially, Guantánamo is an interrogation chamber.
Most crucially, it brings another person into the case.
Most crucially, it changed the structure of work.
Most crucially, he has been a player, too.
Most crucially, he made them good enough, cheaply enough.
Most crucially, Detroit are taking care of the football.
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Since I tried Ludwig back in 2017, I have been constantly using it in both editing and translation. Ever since, I suggest it to my translators at ProSciEditing.

Justyna Jupowicz-Kozak
CEO of Professional Science Editing for Scientists @ prosciediting.com